physics.chem-ph · 2026-09-28 · No. 127
Chemical Physics, 2026-09-28.
1 new papers in physics.chem-ph. Titles, authors,
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01 — The papers
1 entries-
01
Scaling Density Functional Theory with Gaussian Splatting
Andrés Guzmán-Cordero, Cindy Zhang, Majdi Hassan, Marta Skreta, Kirill Neklyudov, Matija Medvidović
physics.chem-ph · cond-mat.mtrl-sci · cs.LG · physics.comp-ph
Density functional theory (DFT) strikes a practical balance between accuracy and computational cost in many problems of computational chemistry and materials science. However, many DFT calculations are limited by fixed atom-centered basis sets, which dictate how accuracy and cost scale with system size. We propose Gaussian Splatting for Density Functional Theory (GS-DFT), which represents molecular orbitals as a cloud of Gaussians whose...
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